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Bond was best known for his work as a child actor for two different nonconsecutive periods on Our Gang (Little Rascals) comedies, and also for being the first actor to portray the role of "Superman`s pal" Jimmy Olsen on screen.

Bond got his start in 1931 at the age of five when a talent scout for Hal Roach studios approached him as he was leaving a Dallas cinema with his mother. The scout asked him if he would like to act in films because he "had a great face" and set up an appointment with Hal Roach in Los Angeles. Hal Roach was gathering new talent for his popular Our Gang comedies. Bond`s grandmother Jane Quin Sauter volunteered to drive the boy to L.A. by motor car. This occurred in the spring of 1931, in the depth of the Great Depression. It proved to be a grueling journey, punctuated by flash floods and encounters with tarantulas, on mostly dirt roads from Dallas to L.A.

Bond was hired at Hal Roach Studios for the Our Gang series in the summer of 1931 to begin work that upcoming fall, at around the same time as George "Spanky" McFarland was hired. Bond worked in Our Gang for two years, alternately appearing as a supporting character and a background actor. His speaking roles increased by 1934, including his most substantive role to this point as the gang`s band conductor in Mike Fright (1934). In late 1934, Bond left the series and returned to public school, still earning periodic bit parts in Hollywood productions.

After leaving the gang for the first time, Bond also worked as a voice actor, most notably in several of Tex Avery`s Merrie Melodies cartoons for Warner Bros. His best known voice role was as the speaking voice of "Owl Jolson" in Tex Avery`s 1936 Merrie Melodies cartoon, I Love to Singa.

Bond returned to Our Gang on a recurring basis late in 1936, when Roach hired him to play "Butch", the neighborhood bully. Bond`s first short as Butch was Glove Taps, filmed in 1936 and released in 1937. Besides filling the role of the archetypal Our Gang bully, the Butch character also regularly competed with meek Alfalfa (Carl Switzer) for the affections of his sweetheart Darla (Darla Hood). While an Our Ganger, Bond appeared in a number of outside films, such as those featuring fellow Hal Roach Studios comedians Charley Chase and Laurel and Hardy.

As Butch, Bond remained with Our Gang an additional three years, staying with the series when it moved to Metro-Goldwyn-Mayer in 1938. His final Our Gang short, Bubbling Troubles, was shot in late 1939 and released in 1940; Bond continued ot work in other MGM productions following his departure from Our Gang. In total, Tommy Bond appeared in 27 Our Gang shorts - 13 as "Tommy" and 14 as "Butch".

After serving in the U.S. Navy during World War II, Bond returned to acting ,and appeared in a handful of East Side Kids, and Gas House Kids features alongside former on-screen rival Carl Switzer. In the late 1940s, Bond became the first actor to portray cub news photographer Jimmy Olsen in two Superman film serials, Superman (1948) and Atom Man vs. Superman (1950). He also appeared as Joey Pepper in several installments of the Five Little Peppers serial.

In 1951, Bond graduated from college and quit acting to stay in show business on the other side of the camera in television directing and production, and worked with individuals such as Norman Lear, George Schlatter, and many others. He worked at Metromedia owned Channel 11, KTTV (now owned and opera